Authors:
T. KanekoNiigata University Department of Chemistry, Faculty of Science Niigata 950-2181 Japan

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S. OnoNiigata University Department of Chemistry, Faculty of Science Niigata 950-2181 Japan

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S. GotoNiigata University Department of Chemistry, Faculty of Science Niigata 950-2181 Japan

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H. HabaJapan Atomic Energy Research Institute Advanced Science Research Center Tokai-mura, Ibaraki 319-1195 Japan

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M. AsaiJapan Atomic Energy Research Institute Advanced Science Research Center Tokai-mura, Ibaraki 319-1195 Japan

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K. TsukadaJapan Atomic Energy Research Institute Advanced Science Research Center Tokai-mura, Ibaraki 319-1195 Japan

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Y. NagameJapan Atomic Energy Research Institute Advanced Science Research Center Tokai-mura, Ibaraki 319-1195 Japan

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H. KudoNiigata University Department of Chemistry Niigata 950-2181 Japan

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Abstract  

An isothermal chromatographic apparatus was developed for the on-line experiments of super heavy elements in gas phase. As a model of Rf, we investigated the gas phase chemistry of Zr and Hf chlorides. The dependence of the reaction efficiency on temperature was examined. It was found that about 80% of Zr and Hf reacted with chlorinating gas at 900 °C. Adsorption enthalpies of Zr and Hf chlorides were deduced from the isothermal chromatograph by the Monte Carlo simulation based on the microscopic model proposed by Zvára.

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Journal of Radionalytical and Nuclear Chemistry
Language English
Size A4
Year of
Foundation
1968
Volumes
per Year
1
Issues
per Year
12
Founder Akadémiai Kiadó
Founder's
Address
H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
Publisher Akadémiai Kiadó
Springer Nature Switzerland AG
Publisher's
Address
H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
CH-6330 Cham, Switzerland Gewerbestrasse 11.
Responsible
Publisher
Chief Executive Officer, Akadémiai Kiadó
ISSN 0236-5731 (Print)
ISSN 1588-2780 (Online)

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