First results studying the transmutation of 129I, 237Np, 238Pu, and 239Pu in the irradiation of an extended natU/Pb-assembly with 2.52 GeV deuterons

M. Krivopustov; A. Pavliouk; A. Kovalenko; I. Mariin; A. Elishev; J. Adam; A. Kovalik; Yu. Batusov; V. Kalinnikov; V. Brudanin; P. Chaloun; V. Tsoupko-Sitnikov; A. Solnyshkin; V. Stegailov; Sh. Gerbish; O. Svoboda; Z. Dubnicka; M. Kala; M. Kloc; A. Krasa; A. Kugler; M. Majerle; V. Wagner; R. Brandt; W. Westmeier; H. Robotham; K. Siemon; M. Bielewicz; S. Kilim; M. Szuta; E. Strugalska-Gola; A. Wojeciechowski; S. Hashemi-Nezhad; M. Manolopoulou; M. Fragopolou; S. Stoulos; M. Zamani-Valasiadou; S. Jokic; K. Katovsky; O. Schastny; I. Zhuk; A. Potapenko; A. Safronova; Zh. Lukashevich; V. Voronko; V. Sotnikov; V. Sidorenko; W. Ensinger; H. Severin; S. Batsev; L. Kostov; Kh. Protokhristov; Ch. Stoyanov; O. Yordanov; P. Zhivkov; A. Kumar; M. Sharma; A. Khilmanovich; B. Marcinkevich; S. Korneev; Ts. Damdinsuren; Ts. Togoo; H. Kumawat

doi:10.1007/s10967-007-7265-1

Journal of Radioanalytical and Nuclear Chemistry

Volume/Issue:: Volume 279: Issue 2

First results studying the transmutation of ¹²⁹I, ²³⁷Np, ²³⁸Pu, and ²³⁹Pu in the irradiation of an extended ^natU/Pb-assembly with 2.52 GeV deuterons

Authors:

M. Krivopustov

M. Krivopustov Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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A. Pavliouk

A. Pavliouk Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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A. Kovalenko

A. Kovalenko Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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I. Mariin

I. Mariin Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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A. Elishev

A. Elishev Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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J. Adam

J. Adam Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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A. Kovalik

A. Kovalik Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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Yu. Batusov

Yu. Batusov Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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V. Kalinnikov

V. Kalinnikov Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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V. Brudanin

V. Brudanin Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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P. Chaloun

P. Chaloun Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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V. Tsoupko-Sitnikov

V. Tsoupko-Sitnikov Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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A. Solnyshkin

A. Solnyshkin Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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V. Stegailov

V. Stegailov Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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Sh. Gerbish

Sh. Gerbish Joint Institute for Nuclear Research Joliot-Curie 6 141980 Dubna Russia

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O. Svoboda

O. Svoboda Nuclear Physics Institute Řež near Praha Czech Republic

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Z. Dubnicka

Z. Dubnicka Nuclear Physics Institute Řež near Praha Czech Republic

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M. Kala

M. Kala Nuclear Physics Institute Řež near Praha Czech Republic

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M. Kloc

M. Kloc Nuclear Physics Institute Řež near Praha Czech Republic

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A. Krasa

A. Krasa Nuclear Physics Institute Řež near Praha Czech Republic

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A. Kugler

A. Kugler Nuclear Physics Institute Řež near Praha Czech Republic

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M. Majerle

M. Majerle Nuclear Physics Institute Řež near Praha Czech Republic

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V. Wagner

V. Wagner Nuclear Physics Institute Řež near Praha Czech Republic

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R. Brandt

R. Brandt Philipps-University Kernchemie, Chemistry Department 35032 Marburg Germany

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W. Westmeier

W. Westmeier

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H. Robotham

H. Robotham Dr. Westmeier GmbH 35085 Ebsdorfergrund Germany

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K. Siemon

K. Siemon Dr. Westmeier GmbH 35085 Ebsdorfergrund Germany

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M. Bielewicz

M. Bielewicz Institute of Atomic Energy 05-400 Otwock-Swierk near Warsaw Poland

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S. Kilim

S. Kilim Institute of Atomic Energy 05-400 Otwock-Swierk near Warsaw Poland

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M. Szuta

M. Szuta Institute of Atomic Energy 05-400 Otwock-Swierk near Warsaw Poland

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E. Strugalska-Gola

E. Strugalska-Gola Institute of Atomic Energy 05-400 Otwock-Swierk near Warsaw Poland

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A. Wojeciechowski

A. Wojeciechowski Institute of Atomic Energy 05-400 Otwock-Swierk near Warsaw Poland

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S. Hashemi-Nezhad

S. Hashemi-Nezhad University of Sydney School of Physics, A28 NSW 2006 Australia

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M. Manolopoulou

M. Manolopoulou Aristotle University School of Physics Thessaloniki 54124 Greece

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M. Fragopolou

M. Fragopolou Aristotle University School of Physics Thessaloniki 54124 Greece

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S. Stoulos

S. Stoulos Aristotle University School of Physics Thessaloniki 54124 Greece

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M. Zamani-Valasiadou

M. Zamani-Valasiadou Aristotle University School of Physics Thessaloniki 54124 Greece

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S. Jokic

S. Jokic Vinca Institute of Nuclear Science Belgrad Serbia

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K. Katovsky

K. Katovsky Czech Technical University Praha Czech Republic

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O. Schastny

O. Schastny Czech Technical University Praha Czech Republic

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I. Zhuk

I. Zhuk Joint Institute of Power and Nuclear Research, Sosny 220109 Minsk Belarus

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A. Potapenko

A. Potapenko Joint Institute of Power and Nuclear Research, Sosny 220109 Minsk Belarus

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A. Safronova

A. Safronova Joint Institute of Power and Nuclear Research, Sosny 220109 Minsk Belarus

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Zh. Lukashevich

Zh. Lukashevich Joint Institute of Power and Nuclear Research, Sosny 220109 Minsk Belarus

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V. Voronko

V. Voronko Kharkov Institute of Physics and Technology Kharkov Ukraine

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V. Sotnikov

V. Sotnikov Kharkov Institute of Physics and Technology Kharkov Ukraine

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V. Sidorenko

V. Sidorenko Kharkov Institute of Physics and Technology Kharkov Ukraine

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W. Ensinger

W. Ensinger Technical University Analytical Chemistry, FB 11 64287 Darmstadt Germany

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H. Severin

H. Severin Technical University Analytical Chemistry, FB 11 64287 Darmstadt Germany

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S. Batsev

S. Batsev Institute of Nuclear Research and Nuclear Energy Sofia Bulgaria

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L. Kostov

L. Kostov Institute of Nuclear Research and Nuclear Energy Sofia Bulgaria

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Kh. Protokhristov

Kh. Protokhristov Institute of Nuclear Research and Nuclear Energy Sofia Bulgaria

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Ch. Stoyanov

Ch. Stoyanov Institute of Nuclear Research and Nuclear Energy Sofia Bulgaria

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O. Yordanov

O. Yordanov Institute of Nuclear Research and Nuclear Energy Sofia Bulgaria

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P. Zhivkov

P. Zhivkov Institute of Nuclear Research and Nuclear Energy Sofia Bulgaria

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A. Kumar

A. Kumar University of Rajastan Jaipur India

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M. Sharma

M. Sharma University of Rajastan Jaipur India

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A. Khilmanovich

A. Khilmanovich Stepanov Institute of Physics Minsk Belarus

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B. Marcinkevich

B. Marcinkevich Stepanov Institute of Physics Minsk Belarus

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S. Korneev

S. Korneev Stepanov Institute of Physics Minsk Belarus

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Ts. Damdinsuren

Ts. Damdinsuren National University Ulaanbaatar Mongolia

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Ts. Togoo

Ts. Togoo National University Ulaanbaatar Mongolia

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H. Kumawat

H. Kumawat Bhabha Atomic Research Center Mumbai 400085 India

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Pages:: 567–584

Online Publication Date:: 28 Sep 2008

Publication Date:: 01 Feb 2009

Article Category:: Research Article

DOI:: https://doi.org/10.1007/s10967-007-7265-1

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Abstract

An extended U/Pb-assembly was irradiated with an extracted beam of 2.52 GeV deuterons from the Nuclotron accelerator of the Laboratory of High Energies within the JINR in Dubna, Russia. The lay-out of this experiment and first results are reported. The Pb-target (diameter 8.4 cm, length 45.6 cm) is surrounded by a ^natU-blanket (206.4 kg) and used for transmutation studies of hermetically sealed radioactive samples of ¹²⁹I, ²³⁷Np, ²³⁸Pu and ²³⁹Pu. Estimates of transmutation rates were obtained as result of measurements of gamma-activities of the samples. Information about the spatial and energy distribution of neutrons in the volume of the lead target and the uranium blanket was obtained with sets of activation threshold detectors (Al, Y and Au) and solid state nuclear track detectors (SSNTD). An electronic ³He neutron detector was tested on-line. A comparison of experimental data with theoretical model calculations using the MCNPX program was performed yielding satisfactory results.

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Journal of Radioanalytical and Nuclear Chemistry

Print ISSN:: 0236-5731

Online ISSN:: 1588-2780

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Journal of Radionalytical and Nuclear Chemistry
Language	English
Size	A4
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