Authors:
Li Gaoliang China Institute of Atomic Energy, Beijing, 102413 China

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He Hui China Institute of Atomic Energy, Beijing, 102413 China

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Zheng Weifang China Institute of Atomic Energy, Beijing, 102413 China

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Tang Hongbin China Institute of Atomic Energy, Beijing, 102413 China

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Li Huirong China Institute of Atomic Energy, Beijing, 102413 China

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Lan Tian China Institute of Atomic Energy, Beijing, 102413 China

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Liu Xiechun China Institute of Atomic Energy, Beijing, 102413 China

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Zhang Hu China Institute of Atomic Energy, Beijing, 102413 China

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Yang He China Institute of Atomic Energy, Beijing, 102413 China

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Luo Fangxiang China Institute of Atomic Energy, Beijing, 102413 China

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Xiao Songtao China Institute of Atomic Energy, Beijing, 102413 China

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Ye Guoan China Institute of Atomic Energy, Beijing, 102413 China

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Abstract  

Oxidation of Pu(III) in 1 bp solution to Pu(IV) was studied using the salt-free oxidant N2O4. It was proved that the reductants N,N-dimethylhydroxylamine (DMHAN) and monomethyl-hydrazine (MMH) present in 1 bp solution of CIAE-APOR process can be oxidized and removed from the solutions also by N2O4 before the oxidation of Pu(III). The effects of the acidity, the temperature and the amount of N2O4 added on the oxidation of DMHAN and MMH were studied.

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Journal of Radionalytical and Nuclear Chemistry
Language English
Size A4
Year of
Foundation
1968
Volumes
per Year
1
Issues
per Year
12
Founder Akadémiai Kiadó
Founder's
Address
H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
Publisher Akadémiai Kiadó
Springer Nature Switzerland AG
Publisher's
Address
H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
CH-6330 Cham, Switzerland Gewerbestrasse 11.
Responsible
Publisher
Chief Executive Officer, Akadémiai Kiadó
ISSN 0236-5731 (Print)
ISSN 1588-2780 (Online)