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Hernane T. Barcelos
Hernane T. Barcelos
Science and Technology of Goiás, Federal Institute of Education, Goiânia, CP, 74055-110, Brazil
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Luclecia D. Nunes
Luclecia D. Nunes
UFG, University of Goias, CP 131, Goiania, GO, 74001-970, Brazil
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Guilherme W. Tavares
Guilherme W. Tavares
QuiCSI Team, Institute of Chemistry, University of Brasilia, CP 4478, Brasilia, DC, 70904-970, Brazil
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Edesio F. C. Alcantara
Edesio F. C. Alcantara
UFG, University of Goias, CP 131, Goiania, GO, 74001-970, Brazil
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Alexandre G. S. Prado
Alexandre G. S. Prado
QuiCSI Team, Institute of Chemistry, University of Brasilia, CP 4478, Brasilia, DC, 70904-970, Brazil
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Abstract
Silica gel was modified by silanization reaction followed by functionalization of histamine in a heterogeneous route. These materials were characterized by elementary nitrogen and chloride analyses, porosity, thermogravimetry, and infrared. The functionalized surface adsorbed Cu(II), Co(II), Ni(II), and Zn(II) ions in an aqueous solution at 25 °C. The isotherms of adsorption are in accordance with Langmuir model and the surface presented a great potential to form complexes metal-surface in the chemical reason of 1:1.
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1. Gao, B, Gao, Y, Li, Y. Preparation and chelation adsorption property of composite chelating material poly(amidoxime)/SiO2 towards heavy metal ions. Chem Engin J. 2010;158: 3 542–549. .
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2. Prado, AGS, Moura, AO, Andrade, RDA, Pescara, IC, Ferreira, VSF, Oliveira, AHA, Okino, EYA, Zara, LF. Application of Brazilian sawdust samples for chromium removal from tannery wastewater. J Therm Anal Calorim. 2010;99: 2 681–687. .
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3. Quintanilla, DP, Hierro, I, Fajardo, M, Sierra, I. 2-Mercaptothiazoline modified mesoporous silica for mercury removal from aqueous media. J Hazard Mater. 2006;134: 1–3 245–256. .
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4. Pereira, AS, Ferreira, G, Caetano, L, Castro, RSD, Santos, A, Padilha, PM, Castro, GR. 4-amine-2-mercaptopyrimidine modified silica gel applied in Cd(II) and Pb(II) extraction from an aqueous medium. Polish J Chem Technol. 2010;12: 1 7–11. .
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5. Wan Ngah, WS, Hanafiah, MAKM. Removal of heavy metal ions from wastewater by chemically modified plant wastes as adsorbents: a review. Bioresour Technol. 2008;99: 10 3935–3948. .
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6. Prado, GS, Moura, AO, Holanda, MS, Carvalho, TO, Andrade, RDA, Pescara, IC, Oliveira, AHA, Okino, EYA, Pastore, TCM, Silva, DJ, Zara, LF. Thermodynamic aspects of the Pb adsorption using Brazilian sawdust samples: removal of metal ions from battery industry wastewater. Chem Engin J. 2010;160: 2 549–555. .
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7. Goswani, A, Singh, AK. Silica gel functionalized with resacetophenone: synthesis of a new chelating matrix and its application as metal ion collector for their flame atomic absorption spectrometric determination. Anal Chim Acta. 2002;454: 2 229–240. .
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8. Evangelista, SM, Oliveira, E, Castro, GR, Zara, LF, Prado, AGS. Hexagonal mesoporous silica modified with 2-mercaptothiazoline for removing mercury from water solution. Surf Sci. 2007;601: 10 2194–2202. .
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9. Skoog, DA, West, DM, Holler, FJ. Fundamentals of analytical chemistry. Florida: CRC; 2003.
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10. Alcântara, EFC, Faria, AE, Rodrigues, DV, Evangelista, SM, Oliveira, E, Zara, LF, Rabelo, D, Prado, AGS. Modification of silica gel by attachment of 2-mercaptobenzimidazole for use in removing Hg(II) from aqueous media: a thermodynamic approach. J Colloid Interface Sci. 2007;311: 1 1–7. .
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11. Prado, AGS, Miranda, BS, Jacintho, GVM. Interaction of indigo carmine dye with silica modified with humic acids at solid/liquid interface. Surf Sci. 2003;542: 3 276–282. .
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12. Prado, AGS, Sales, JAA, Carvalho, RM, Rubim, JC, Airoldi, C. Immobilization of 5-amino-1,3,4-thiadiazole-thiol onto silica gel surface by heterogeneous and homogeneous routes. J Non-Crystal Sol. 2004;333: 1 61–67. .
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13. Cestari, AR, Airoldi, C. Chemisorption on thiol-silicas: divalent cations as a function of pH and primary amines on thiol-mercury adsorbed. J Colloid Interf Sci. 1997;195:338–342. .
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14. Arakaki, LNH, Augusto Filha, VLS, Sousa, KS, Aguiar, FP, Fonseca, MG, Espínola, JGP. Silica gel ethyleneimine and its adsorption capacity for divalent Pb, Cd, and Hg. Thermochim Acta. 2006;440: 2 176–180. .
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15. Sales, JAA, Prado, AGS, Airold, C. Thermodynamic data for divalent cations onto new modified glycidoxy silica surface at solid/liquid interface. J Therm Anal Calorim. 2002;70: 1 135–141. .
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16. Augusto Filha, VLS, Silva, OG, Costa, JR, Wanderley, AF, Fonseca, MG, Arakaki, LNH. Interaction of divalent cations Zn, Cd and Hg on surface of silica gel with aminoethanethiol as evaluated by calorimetric titration. J Therm Anal Calorim. 2007;87: 3 621–625. .
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17. Torres, JD, Faria, EA, Prado, AGS. Thermodynamic studies of the interaction at the solid/liquid interface between metal ions and cellulose modified with ethylenediamine. J Hazard Mater. 2006;129: 1–3 239–243. .
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| Journal of Thermal Analysis and Calorimetry | |
|---|---|
| Language | English |
| Size | A4 |
| Year of Foundation |
1969 |
| Volumes per Year |
1 |
| Issues per Year |
24 |
| Founder | Akadémiai Kiadó |
| Founder's Address |
H-1117 Budapest, Hungary 1516 Budapest, PO Box 245. |
| Publisher | Akadémiai Kiadó Springer Nature Switzerland AG |
| Publisher's Address |
H-1117 Budapest, Hungary 1516 Budapest, PO Box 245. CH-6330 Cham, Switzerland Gewerbestrasse 11. |
| Responsible Publisher |
Chief Executive Officer, Akadémiai Kiadó |
| ISSN | 1388-6150 (Print) |
| ISSN | 1588-2926 (Online) |
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