A series of samples of the type Ni0.65Zn0.35CuxFe2−xO4 (x=0, 0.1, 0.2, 0.3, 0.4 and 0.5) were prepared by means of a ceramic technique. The existence of a single phase was confirmed in X-ray studies. The dielectric constantK and dielectric lossD were measured at different temperatures at a frequency of 1 kHz. The pronounced increase in the dielectric constant at the transition temperature is due to the phase transformation from the ferrimagnetic to the paramagnetic state. The decrease in the dielectric loss with temperature is due to the reduction in the relaxation time of the hopping electrons and holes. The Tawfik constant was calculated in the ferrimagnetic state and was found to be correlated to the dielectric constant.