A series of coprecipitates of basic cobalt carbonate and hydrated titanium oxide were investigated by TG and DTA up to 1000°. In the absence of water and CO2, an oxide system is obtained consisting of Co3O4 and TiO2, from which cobalt metatitanate is first formed; from the latter, depending on the presence of TiO2 or Co3O4 in the system, the dititanate or the orthotitanate is formed. IR absorption and X-ray spectra and TG and DTA curves prove that the double oxides of cobalt and titanium are obtained in this manner at temperatures lower than in other methods; this gives them useful properties for practical applications.