Reaction Kinetics, Mechanisms and Catalysis
Volume/Issue:
Volume 103: Issue 1
Influence of Pd on FeAlPO-5 zeolite in the catalytic reduction of N2O with methane
Authors:
Dang-guo Cheng Department of Chemical and Biological Engineering, Zhejiang University, 38 Zheda Road, Hangzhou 310027, China

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Cheng Zhu Department of Chemical and Biological Engineering, Zhejiang University, 38 Zheda Road, Hangzhou 310027, China

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Xiaoxu Zhao Department of Chemical and Biological Engineering, Zhejiang University, 38 Zheda Road, Hangzhou 310027, China

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Fengqiu Chen Department of Chemical and Biological Engineering, Zhejiang University, 38 Zheda Road, Hangzhou 310027, China

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Xiaoli Zhan Department of Chemical and Biological Engineering, Zhejiang University, 38 Zheda Road, Hangzhou 310027, China

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Pages:
219–226
Online Publication Date:
01 Apr 2011
Publication Date:
01 Jun 2011
Article Category:
Research Article
DOI:
https://doi.org/10.1007/s11144-011-0304-5
Keywords:
FeAlPO-5; Methane; Catalytic reduction; Nitrous oxide; Palladium
Restricted access

Abstract

Pd/FeAlPO-5 zeolites with different Pd loading were prepared and characterized by N2 physisorption, XRD and H2-TPR. The results indicate that Pd addition has little influence on the textural structure of FeAlPO-5 zeolites. The TPR profiles of zeolites show the peak temperatures related with the reduction of Fe(III) and subsurface Pd species decrease with the increase of Pd content, suggesting the existence of interactions between Fe and Pd. The Pd/FeAlPO-5 catalysts were tested in the catalytic reduction of N2O with methane and show a better low-temperature activity in comparison with FeAlPO-5. The improved activity of Pd/FeAlPO-5 can be ascribed to the synergic effect between noble metal and iron species.

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Cover Reaction Kinetics, Mechanisms and Catalysis
Reaction Kinetics, Mechanisms and Catalysis
Print ISSN:
1878-5190
Online ISSN:
1878-5204

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Reaction Kinetics, Mechanisms and Catalysis
Language English
Size B5
Year of
Foundation		 1974
Volumes
per Year		 1
Issues
per Year		 6
Founder Akadémiai Kiadó
Founder's
Address		 H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
Publisher Akadémiai Kiadó
Springer Nature Switzerland AG
Publisher's
Address		 H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
CH-6330 Cham, Switzerland Gewerbestrasse 11.
Responsible
Publisher		 Chief Executive Officer, Akadémiai Kiadó
ISSN 1878-5190 (Print)
ISSN 1878-5204 (Online)

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