Reaction Kinetics, Mechanisms and Catalysis
Volume/Issue:
Volume 104: Issue 2
Thermodynamic analysis of the cluster size evolution in catalyst preparation by deposition–precipitation
Authors:
Dmitry Yu. Murzin Laboratory of Industrial Chemistry and Reaction Engineering, Åbo Akademi University, Biskopsgatan 8, Turku/Åbo, Finland

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Olga A. Simakova Laboratory of Industrial Chemistry and Reaction Engineering, Åbo Akademi University, Biskopsgatan 8, Turku/Åbo, Finland

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Irina L. Simakova Boreskov Institute of Catalysis, Novosibirsk, Russia

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Valentin N. Parmon Boreskov Institute of Catalysis, Novosibirsk, Russia

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Pages:
259–266
Online Publication Date:
17 Aug 2011
Publication Date:
01 Dec 2011
Article Category:
Research Article
DOI:
https://doi.org/10.1007/s11144-011-0363-7
Keywords:
Thermodynamics; Cluster size; Growth; Catalyst preparation; Deposition-precipitation
Restricted access

Abstract

Several gold catalysts supported on various inorganic supports with different point zero charge (pzc) were prepared by deposition–precipitation with urea (DPU). A thermodynamic model accounting for cluster evolution was advanced. The key element in the model is the dependence of the interfacial energy on the relative approach to pzc during DP. Experimental data were compared with the model, showing a possibility to utilize the theoretical approach to predict the cluster size.

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Cover Reaction Kinetics, Mechanisms and Catalysis
Reaction Kinetics, Mechanisms and Catalysis
Print ISSN:
1878-5190
Online ISSN:
1878-5204

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Reaction Kinetics, Mechanisms and Catalysis
Language English
Size B5
Year of
Foundation		 1974
Volumes
per Year		 1
Issues
per Year		 6
Founder Akadémiai Kiadó
Founder's
Address		 H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
Publisher Akadémiai Kiadó
Springer Nature Switzerland AG
Publisher's
Address		 H-1117 Budapest, Hungary 1516 Budapest, PO Box 245.
CH-6330 Cham, Switzerland Gewerbestrasse 11.
Responsible
Publisher		 Chief Executive Officer, Akadémiai Kiadó
ISSN 1878-5190 (Print)
ISSN 1878-5204 (Online)

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