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Journal of Radioanalytical and Nuclear Chemistry
Authors:
M. Krivopustov
,
J. Adam
,
V. Bradnova
,
R. Brandt
,
V. Butsev
,
P. Golubev
,
V. Kalinnikov
,
J. Karachuk
,
B. Kulakov
,
E.-J. Langrock
,
G. Modolo
,
M. Ochs
,
R. Odoj
,
A. Premyshev
,
V. Pronskich
,
Th. Schmidt
,
V. Stegailov
,
J. Wan
, and
V. Zupko-Sitnikov

Abstract  

First experiments on the transmutation of long-lived129I and237Np using relativistic protons of 3.7 GeV are described. Relativistic protons generate in extended Pb-targets substancial neutron fluences. These neutrons get moderated in paraffin and are used for transmutation as follows:129I(n,)130I and237Np(n,)238Np . The isotopes130I (T 1/2-12.36 h) and238Np (T 1/2=2.117 d) were identified radiochemically. One can estimate the transmutation cross-section (n,) in the given neutron field as (129I(n,))=(10±2)b and (237Np(n,))=(140±30)b The experiments were carried out in November 1996 at the Synchrophasotron, LHE, Dubna, Russia. The investigation has been performed at the Laboratory of High Energies, JINR, Dubna.

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Journal of Radioanalytical and Nuclear Chemistry
Authors:
B. Bisplinghoff
,
V. Bradnova
,
R. Brandt
,
K. Dwivedi
,
V. Butsev
,
E. Friedlander
,
S. Gosh
,
Guo Shi-Lun
,
M. Heck
,
Jin Huimin
,
M. Krivopustov
,
B. Kulakov
,
C. Laue
,
L. Lerman
,
Th. Schmidt
,
A. Sosnin
, and
Wang Yu-Lan

Abstract  

An extended Cu-target was irradiated with 22 and 44 GeV carbon ions for about 11.3 and 14.7 hours, respectively. The upper side of the target was in contact with a paraffin-block for the moderation of secondary neutrons. Small holes in the moderator were filled with either lanthanum salts or uranium oxide. The reaction
\documentclass{aastex} \usepackage{amsbsy} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{bm} \usepackage{mathrsfs} \usepackage{pifont} \usepackage{stmaryrd} \usepackage{textcomp} \usepackage{upgreek} \usepackage{portland,xspace} \usepackage{amsmath,amsxtra} \pagestyle{empty} \DeclareMathSizes{10}{9}{7}{6} \begin{document} $${}^{139}La(n,\gamma ){}^{140}La\mathop \to \limits^{\beta - }$$ \end{document}
was studied via the decay of140La(40h) using radiochemical methods, as has been published. The reaction
\documentclass{aastex} \usepackage{amsbsy} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{bm} \usepackage{mathrsfs} \usepackage{pifont} \usepackage{stmaryrd} \usepackage{textcomp} \usepackage{upgreek} \usepackage{portland,xspace} \usepackage{amsmath,amsxtra} \pagestyle{empty} \DeclareMathSizes{10}{9}{7}{6} \begin{document} $${}^{238}U(n,\gamma )^{239} U\mathop \to \limits^{\beta - } {}^{239}Np\mathop \to \limits^{\beta - }$$ \end{document}
was studied via the decay of239Np(2.3 d) as well as the reaction U(n,f) using radiochemical methods. In addition, solid state nuclear track detectors were used for fission studies in gold. The yields for the formation of (n,) products agree essentially with other experiments on extended targets carried out at the Dubna Synchrophasotron (LHE, JINR). To a first approximation, the breeding rate of (n, ) products doubles when the carbon energy increases from 22 to 44 GeV. If, however, results at 44 GeV are compared in detail to those at 22 GeV, we observe an excess of (37±9)% in the experimentally observed239Np-breeding rate over theoretical estimations. Experiments using solid state nuclear track detectors give similar results. We present a conception for the interpretation of this fact: There is the evident connection between anomalies we observe in the yield of secondary particles in relativistic heavy ion interactions above a total energy of approximately 30–35 GeV and increased yield of neutrons in this energy region.
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