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  • Author or Editor: N. Yanase x
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Abstract  

The concentration of pore water uranium in six sediments from oligotrophic, mesotrophic, acidotrophic and dystrophic lakes was measured by inductively coupled plasma-mass spectrometry. Profiles of pore water U can be divided into two groups such as low (17±7 ng/l) and high concentration (69±30 ng/l). These values were 1–2 orders of magnitude higher than that of lake waters (6±4 ng/l) due to the release of U from the sediments by decomposition of organic materials. Variations in pore water U concentrations seem to relate to the differences in pore water pH, the association forms, and their contents of U in the lake sediments.

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Abstract  

Surface soil samples (0–1 cm) were collected to understand the role of hot particle (HP) in migration of radionuclide approximately 11 years after the Chernobyl accident. Three types of HPs were found by the analyses using alpha-track technique and scanning electron microscopy/energy dispersive X-ray spectrometer (SEM/EDX). The dissolution of HPs has been affected by the existing type of HPs. Six-stage sequential selective extraction procedure was carried out to define the chemical forms of uranium, 241Am and 137Cs. The chemical form of radionuclides in surface soil is significantly different between the west and the north traces of radioactive plumes approximately 11 years after the accident.

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